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Evaluation of Monochloramine and Free Chlorine Penetration in a Drinking Water Storage Tank Sediment Using Microelectrodes

Metadata Updated: November 12, 2020

Sediment accumulation in water storage tanks may protect microorganisms from disinfectant exposure, causing water quality degradation. However, microbial activity and disinfectant penetration within water storage sediment remains largely uncharacterized. This study evaluated monochloramine and free chlorine penetration into a 2-cm (20,000 µm) deep drinking water storage tank sediment using microelectrodes. The sediment was successively exposed to 4-months monochloramine, 2-months free chlorine, and 2-months monochloramine. Temporal monochloramine, free chlorine, dissolved oxygen (DO), pH, ammonium, nitrite, and nitrate profiles were acquired using microelectrodes. Results showed that complete monochloramine or free chlorine penetration was not observed. Likewise, DO never fully penetrated the sediment, progressing inward with time to a maximum depth of 10,000 µm and indicating microbial activity remained during the entire 8 months. Decreasing ammonium and increasing nitrate concentrations, with minimal nitrite accumulation, further demonstrated microbial activity and indicated complete sediment nitrification. There was measurable ammonium, nitrite, and nitrate during free chlorine application and nitrification activity gradually resumed upon a switch back to monochloramine. These findings suggest that periodic sediment removal from drinking water storage facilities is desirable to remove potentially protected environments for microorganisms.

This dataset is associated with the following publication: Liu, H., D. Wahman, and J. Pressman. Evaluation of Monochloramine and Free Chlorine Penetration in a Drinking Water Storage Tank Sediment Using Microelectrodes. ENVIRONMENTAL SCIENCE & TECHNOLOGY. American Chemical Society, Washington, DC, USA, 53(16): 9352-9360, (2019).

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Public: This dataset is intended for public access and use. License: See this page for license information.

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References

https://doi.org/10.1021/acs.est.9b01189

Dates

Metadata Created Date November 12, 2020
Metadata Updated Date November 12, 2020

Metadata Source

Harvested from EPA ScienceHub

Additional Metadata

Resource Type Dataset
Metadata Created Date November 12, 2020
Metadata Updated Date November 12, 2020
Publisher U.S. EPA Office of Research and Development (ORD)
Maintainer
Identifier https://doi.org/10.23719/1503400
Data Last Modified 2019-02-11
Public Access Level public
Bureau Code 020:00
Schema Version https://project-open-data.cio.gov/v1.1/schema
Harvest Object Id 9be075d8-a006-4fbc-87ea-c6c4f857fa3e
Harvest Source Id 04b59eaf-ae53-4066-93db-80f2ed0df446
Harvest Source Title EPA ScienceHub
License https://pasteur.epa.gov/license/sciencehub-license.html
Program Code 020:096
Publisher Hierarchy U.S. Government > U.S. Environmental Protection Agency > U.S. EPA Office of Research and Development (ORD)
Related Documents https://doi.org/10.1021/acs.est.9b01189
Source Datajson Identifier True
Source Hash 5a23261925d3fb71f30da5ec82bcf3a3cbd089aa
Source Schema Version 1.1

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